In the photovoltaic effect a single light quanta (photon) is absorbed by a material, exciting an electron to a higher band, and potentially generating a photocurrent if the sample is gated by external voltage, or has some broken symmetry. We are interested in analogues of this effect in the multi-photon and highly-nonlinear regime. Here photocurrents can be generated by extremely short few-cycle pulses, and even in inversion-symmetric materials if the symmetries of the laser pulse itself are pre-engineered.
We attempt to uncover the attosecond nature of this process and its connection to electron dynamics inside the solid, develop spectroscopy techniques for all-optical detection of currents, and utilizing current measurements for ultrafast spectroscopy of various material properties and phenomena.
Relevant publications:
Neufeld, Hübener, De Giovannini, Rubio, “Tracking electron motion within and outside of Floquet bands from attosecond pulse trains in time-resolved ARPES”, J. Phys.: Cond. Matt. 36, 225401 (2024), Emerging leaders issue.
Neufeld, Hübener, Jotzu, De Giovannini, Rubio, “Band nonlinearity-enabled manipulation of Dirac nodes, Weyl cones, and valleytronics with intense linearly polarized laser”, Nano Lett. 23, 7568 (2023).
Galler, Rubio, Neufeld, “Mapping light-dressed Floquet bands by highly nonlinear optical excitations and valley polarization”, J Phys. Chem. Lett. 14, 11298-11304 (2023).
Neufeld, Tancogne-Dejean, De Giovannini, Hübener, Rubio, “Light-Driven Extremely Nonlinear Bulk Photogalvanic Currents”, Phys. Rev. Lett. 127, 126601 (2021).