Hello! I am Zefei Wu, a Researcher working in the field of experimental condensed matter physics.
My current research focuses on developing ultra-high-quality van der Waals two-dimensional electron systems as a platform for exploring emerging topological and correlated quantum phenomena, while leveraging these fundamental discoveries to develop new quantum devices for future electronics and emerging functionalities.
Web of Science Researcher ID: D-1851-2015
ORCiD: https://orcid.org/0000-0001-7123-9156
E-mail: zefeiw@gmail.com
I. Ultra-high quality 2D electronic systems
⭕ Extraordinary electronic quality in proximity screened graphene
Electronic quality is crucial for probing quantum transport, with GaAlAs heterostructures long holding the record after decades of optimization that pushed mobilities to ~5.7 × 10⁷ cm² V⁻¹ s⁻¹. Graphene has progressed from ~10⁴ cm² V⁻¹ s⁻¹ on Si wafers to ~10⁵ and then ~10⁶ cm² V⁻¹ s⁻¹ in suspended and hBN-encapsulated devices respectively, though its low-temperature mobility has been limited by edge scattering and charge inhomogeneity. In this project, I successfully introduced a proximity screening strategy and fabricated devices with graphite proximity gate positioned just 1 nm from graphene. This approach reduces charge inhomogeneity by nearly two orders of magnitude, enabling quantum mobilities of ~10⁷ cm² V⁻¹ s⁻¹ and record transport mobilities exceeding 10⁸ cm² V⁻¹ s⁻¹. This breakthrough allows phenomena such as Shubnikov–de Haas oscillations and the quantum Hall effect to emerge at ultra-low magnetic fields, providing a powerful platform for exploring phenomena, in previously inaccessible regimes.
Proximity screening greatly enhances electronic quality of graphene,
Nature 644, 646–651 (2025).
⭕ On-device phase-engineering for record-high-mobility 2D semiconductors
Forming good electrical contacts with atomically thin transition metal dichalcogenide semiconductors (TMDSCs) is difficult due to interfacial barriers. This work introduces an approach that uses interfacial local bonding distortion to achieve nearly barrier-free contacts, enabling efficient carrier injection and stable ohmic behavior from room to cryogenic temperatures. The resulting TMDSC transistors demonstrate ultra-low contact resistance (as low as 90 Ω µm, towards the quantum limit), exceptionally record high mobility (up to 358,000 cm²V⁻¹s⁻¹), and excellent cryogenic transport properties. Beyond improving contacts, the method allows local tuning of atomic and electronic structures for advanced TMDSC device engineering.
Bridging the gap between atomically thin semiconductors and metal leads,
⭕ Unconventional quantum Hall effect in high-mobility Q-valley electrons
This work reports quantum transport studies of Q-valley electrons in few-layer transition metal disulfides (TMDs), enabled by high-mobility BN-encapsulated devices with optimized contacts. Pronounced Shubnikov–de Haas oscillations and the onset of quantum Hall plateaus are observed, revealing distinct Zeeman responses: a valley Zeeman effect in odd-layer TMDs and a spin Zeeman effect in even-layer TMDs. These contrasting behaviors arise from the presence or absence of inversion symmetry, which dictates spin–valley coupling at the Q valleys. The results extend the unique spin–valley physics of monolayer TMDs to few-layer systems, providing new insights into multi-valley band structures and unconventional quantum Hall effects.
Even–odd layer-dependent magnetotransport of high-mobility Q-valley electrons in transition metal disulfides,
II. Quantum and topological electron transport in van der Waals 2D electron systems
⭕ Probe the intrinsic valley Hall effect without the need of extrinsic symmetry breaking
Earlier experiments generally realized the valley Hall effect by artificially breaking inversion symmetry through substrate coupling or a dual-gate electric field, or by breaking time-reversal symmetry through valley-selective excitation with circularly polarized light. These studies did not directly establish intrinsic valley transport determined by the material’s own properties. In this work, I report the first experimental observation of intrinsic valley Hall effect (VHE) in odd-layer MoS2 without the need of extrinsic symmetry breaking. Nonlocal transport measurements reveal a cubic scaling of nonlocal resistance with local resistance in monolayer and trilayer devices, consistent with VHE driven by Berry curvatures at inequivalent valleys. The effect persists up to room temperature, with micron-scale valley diffusion lengths. These findings establish odd-layer TMDCs as an ideal platform for topological valley transport and open pathways toward electrically controlled, low-dissipation valleytronics.
Intrinsic valley Hall transport in atomically thin MoS2,
⭕ Electric-field control of the Berry curvature dipole
This work reports the intrinsic nonlinear Hall effect in twisted bilayer graphene (TBG), arising from a Berry curvature dipole within its flatbands. Unlike extrinsic effects caused by disorder scattering in graphene superlattices, the observed second harmonic Hall voltage here directly reflects the intrinsic Berry curvature distribution. Applying a displacement field shifts the Berry curvature hotspots, enabling tunable direction and amplitude of the nonlinear Hall response. These results demonstrate that high-quality TBG serves as a sensitive platform for probing Berry curvature and for potential applications in second harmonic generation and rectification.
Intrinsic nonlinear Hall effect and gate-switchable Berry curvature sliding in twisted bilayer graphene,
Physical Review Letters 131, 066301 (2023) editors' suggestion.
⭕ Detection of correlated quantum phase transitions through topological nonlinear transport measurements
The recently discovered nonlinear Hall effect (NHE) in a few non-interacting topological systems provides a novel mechanism for generating second-harmonic electrical Hall signals under time-reversal-symmetric conditions. In this study, we demonstrate a giant nonlinear Hall effect in twisted WSe2 bilayers, enabled by moiré flat bands and strong electron correlations. At half-filling of the first moiré band, the NHE signal peaks sharply, showing a generation efficiency over two orders of magnitude higher than previously reported materials. The enhancement is closely tied to correlation-driven phenomena, with resistivity data suggesting a mass-diverging continuous Mott transition near the insulating state. These findings highlight how moiré engineering can combine Berry curvature dipoles with interaction effects to generate novel quantum responses and establish NHE as a powerful probe of quantum criticality.
Giant nonlinear Hall effect in twisted bilayer WSe₂,
National Science Review 10, nwac232 (2023). ESI highly cited paper. NSR 2025 "Best Paper Award"
III. Synthesis, Mass Transport, and Emerging Functionalities of van der Waals Materials
⭕ In-situly oxided graphene membrane for high effecient proton transport
This study demonstrates that monolayer graphene oxide (GO) membranes are simultaneously impermeable to gases and highly conductive to protons across the basal plane. Contrary to the common assumption of abundant nanoscale pinholes, micrometer-scale GO areas show no helium leakage while exhibiting proton conductivity nearly two orders of magnitude higher than graphene. The enhanced transport originates from oxygen functional groups that distort the graphene lattice and create abundant active sites for proton passage. These findings highlight how chemical functionalization can be harnessed to boost proton transparency of 2D crystals without sacrificing gas impermeability, offering pathways for advanced proton exchange membranes.
Proton and molecular permeation through the basal plane of monolayer graphene oxide,
Nature Communications 14, 7756 (2023).
⭕ Transfer-free growth of high-quality monolayer graphene
In this work, we report on a simple rapid thermal treatment method for the fast and direct growth of high-quality, large-scale monolayer graphene on a SiO2/Si substrate from solid carbon sources. The stack structure of a solid carbon layer/copper film/SiO2 is adopted. The copper film does not only act as an active catalyst for the carbon precursor but also serves as a “filter” that prevents premature carbon dissolution, and thus, contributes to graphene growth on the SiO2 surface. The produced graphene exhibits a high carrier mobility of up to 3000 cm2 V−1 s−1 at room temperature and standard half-integer quantum oscillations at liquid-helium temperatures.
A fast transfer-free synthesis of high-quality monolayer graphene on insulating substrates by a simple rapid thermal treatment,
Nanoscale 8, 2594-2600 (2016). featured on the cover
⭕ Sliding ferroelectric devices based on marginally twisted 2D semiconductors
Robust room-temperature ferroelectricity was reported in marginally twisted MoS2 heterostructures, arising from broken inversion symmetry and interfacial charge transfer at the twisted bilayer interface. In this work, I contribute marginally twisted bilayer (monolayer+monolayer) MoS₂ ferroelectric devices, which exhibit pronounced hysteresis behavior of the conductivity when tuning the gate voltages (shown in the right figure). It is the first semiconducting sliding ferroelectric field-effect transistor that has ever been reported.
Interfacial ferroelectricity in marginally twisted 2D semiconductors,
Nature Nanotechnology 17, 390–395 (2022).
🔸 Graphene quantum capacitor
🔸Monolayer MoS2 valley Hall transistor
🔸Twisted bilayer WSe2 nonlinear Hall device
🔸Double-layer MoS2 FET with Corbino geometry
🔸Double-layer WSe2 FET with Hall bar geometry
🔸Dark-field optical image of a Hall bar device