My research interests focus on condensed matter theories of strongly correlated electronic systems, especially on frustrated magnetism and its emergent phenomena, phase transitions, disorder effects, and dynamical properties.
Disorder effect in Kitaev spin liquid
Field-induced transitions in classical spin ice
Computational methods in many-body physics
Masahiro O. Takahashi, Wen-Han Kao, Satoshi Fujimoto, and Natalia B. Perkins
npj Quantum Mater. 10, 14 (2025)
Keywords: Kitaev Spin liquid, Impurity, Flux-binding effect
Stabilizing Z2 fluxes in Kitaev spin liquids (KSLs) is crucial for both characterizing candidate materials and identifying Ising anyons. In this study, we investigate the effects of spin-S magnetic impurities embedded in the spin-1/2 KSL. Utilizing exact diagonalization and density matrix renormalization group methods, we examine the impurity magnetization and ground-state flux sector with varying impurity coupling and spin size. Our findings reveal that impurity magnetization exhibits an integer/half-integer spin dependence, which aligns with analytical predictions, and a flux-sector transition from bound-flux to zero-flux occurs at low coupling strengths, independent of the impurity spin. Notably, for spin-3/2 impurities, we observe a reentrant bound-flux sector, which remains stable under magnetic fields. By considering fermionic representations of our spin Hamiltonian, we provide phenomenological explanations for the transitions. Our results suggest a novel way of binding a flux in KSLs, beyond the proposals of vacancies or Kondo impurities.
Vitor Dantas, Wen-Han Kao, and Natalia B. Perkins
Phys. Rev. B 110, 104425 (2024)
Keywords: Kitaev Spin Liquid, Site Dilution, Sound Attenuation
Identifying quantum spin-liquid phases is a formidable challenge due to the lack of long-range order and usually relies on indirect dynamical probes. Among various experimental probes, ultrasound experiments measuring sound attenuation have emerged as a promising avenue to unveil the fractionalization of spins in candidate materials. Yet, the observed behaviors of the Kitaev materials often deviate from the ideal Kitaev model due to the presence of disorder, leading to the emergence of localized modes governing low-energy physics. To provide further insight into the effects of these defect-induced modes on the phonon dynamics, we calculate the sound attenuation coefficient in the site-disordered Kitaev honeycomb model with an applied magnetic field, which breaks the time-reversal symmetry. To obtain a more accurate perspective on the temperature-dependent sound attenuation in this model, the impact of thermally excited fluxes on the disordered system is also analyzed.
Vladislav Poliakov, Wen-Han Kao, and Natalia B. Perkins
Phys. Rev. B 110, 054418 (2024)
Keywords: Yao-Lee model, Site Dilution, Topological Transition
The Yao-Lee (YL) model is an example of exactly solvable spin-orbital models that are generalizations of the original Kitaev honeycomb model with extra local orbital degrees of freedom. Similar to the Kitaev model, both spin and orbital degrees of freedom are effectively represented using sets of three-flavored Majorana fermions. The YL model exhibits a quantum spin liquid ground state with gapped and immobile Z2 fluxes and three-fold degenerate itinerant Majorana fermions. Our work demonstrated that by introducing different time-reversal symmetry (TRS) breaking fields one can split the degeneracy of Majorana fermions and close the gap for some of the bands, thus changing its topology. We calculated a comprehensive topological phase diagram for the YL model by considering various combinations of TRS breaking fields. This investigation revealed the emergence of distinct topological regions, each separated by nodal lines, signifying an evolution in the model's topological properties. We also investigated the impact of vacancies in the system. Our findings revealed that while vacancies modify the low-energy spectrum of the model, their presence has a limited impact on the topological properties of the model, at least for small enough concentrations.
Wen-Han Kao, Gábor B. Halász, and Natalia B. Perkins
Phys. Rev. B 109, 125150 (2024) (Editors' Suggestion)
Keywords: Kitaev Spin Liquid, Site Dilution, STM, Dynamical Correlation Function
We study the dynamical response of vacancy-induced quasiparticle excitations in the site-diluted Kitaev spin liquid with a magnetic field. Due to the flux-binding effect and the emergence of dangling Majorana fermions around each spin vacancy, the low-energy physics is governed by a set of vacancy-induced quasi-zero-energy modes. These localized modes result in unique characteristics of the dynamical spin correlation functions, which intriguingly mimic the single-quasiparticle density of states and further exhibit a quasi-zero-frequency peak. By recognizing the potential observability of these local correlation functions via scanning tunneling microscopy (STM), we show how the STM response is sensitive to the local flux configuration, the magnetic field strength, and the vacancy concentration. Constructing a simple model of the localized modes, we also elucidate how the local correlation functions can be interpreted in terms of the hybridization between these modes.
Wen-Han Kao, Natalia B. Perkins, and Gábor B. Halász
Phys. Rev. Lett. 132, 136503 (2024) (Editors' Suggestion)
Keywords: Kitaev Spin Liquid, Site Dilution, STM, Dynamical Correlation Function
We study the spectroscopic signatures of vacancy-induced Majorana zero modes of the Kitaev spin liquid in the inelastic STM setup. When a clean Kitaev spin liquid is placed between the tip and the substrate, the tunneling barrier involves the flux-excitation gap that leads to a zero-response region. However, in the presence of vacancies, a quasi-zero-energy peak appears in the flux-gap region, and its characteristic voltage and intensity are increased with vacancy concentrations, which can be attributed to the localized nature of vacancy-induced Majorana zero modes. The presence of these Majorana zero modes also makes the single-fermion van Hove singularity visible in the STM response, which represents the energy scale of fractionalized Majorana fermions in the Kitaev spin liquid.
Wen-Han Kao and Natalia B. Perkins
Phys. Rev. B 106, L100402 (2022)
Keywords: Kitaev Spin Ladder, Bond Randomness, Strong-disorder Renormalization Group
We study the Kitaev spin ladder with random couplings by using the real-space renormalization group technique. This model is the minimum model in Kitaev systems that has conserved plaquette fluxes, and its quasi-one-dimensional geometry makes it possible to study the strong-disorder fixed points for both spin- and flux- excitation gaps. In the Ising limit, the behavior of the spin gap is consistent with the familiar random transverse-field Ising chain, but the flux gap is dominated by the y-coupling. In the XX limit, while the x- and y-couplings are renormalized simultaneously, the z-couplings are not renormalized drastically and lead to non-universal disorder criticality at low-energy scales.
Wen-Han Kao and Natalia B. Perkins
Keywords: Kitaev Spin Liquid, Disorder Effect, Thermal Conductivity
Motivated by the emergence of this plethora of 4d and 5d transition metal Kitaev materials and by the fact that some level of disorder is inevitable in real materials, we study how the Kitaev spin liquid responds to various forms of disorder, such as vacancies, impurities, and bond randomness. We argue that the presence of the quenched disorder can lead to the Anderson localization of Majorana fermions and the appearance of Lifshitz tails, and that the disorder effects on the low-energy Majorana modes can be detected in thermal transport. While we find that both the site disorder and the bond randomness suppress the longitudinal thermal conductivity, the low-energy localization is stronger in the case of the site disorder.
Wen-Han Kao, Johannes Knolle, Gábor B. Halász, Roderich Moessner and Natalia B. Perkins
Phys. Rev. X 11, 011034 (2021)
Keywords: Kitaev Spin Liquid, Site Dilution, Specific Heat
We demonstrate that a finite density of random vacancies in the Kitaev model gives rise to a striking pileup of low-energy Majorana modes and reproduces the apparent power-law upturn in the specific heat measurements of H3LiIr2O6. We show numerically that the vacancy effect is readily detectable even at low vacancy concentrations and that it is not very sensitive either to the nature of vacancies or to different flux backgrounds. We also propose a field-induced flux-sector transition where the ground state becomes flux-free for larger fields, resulting in a clear suppression of the low-temperature specific heat.
Wen-Han Kao, Gia-Wei Chern, and Ying-Jer Kao
Phys. Rev. Res. 2, 023046 (2020)
Keywords: Kagome Spin Ice, Kinetic Monte Carlo, Metastability
We study the two-dimensional kagome-ice model derived from a pyrochlore lattice with second- and third-neighbor interactions. The canted moments align along the local ⟨111⟩ axes of the pyrochlore and respond to both in-plane and out-of-plane external fields. We find that the combination of further-neighbor interactions together with the external fields introduces a rich phase diagram with different spin textures. Close to the phase boundaries, metastable “snake” domains emerge with extremely long relaxation time. Our kinetic Monte Carlo analysis of the magnetic-field quench process from saturated state shows unusually slow dynamics. Although the interior spins are almost frozen in snake domains, the spins on the edge are free to fluctuate locally, leading to frequent creation and annihilation of monopole-antimonopole bound states.
Kai-Wen Zhao, Wen-Han Kao, Kai-Hsin Wu, and Ying-Jer Kao
Phys. Rev. E 99, 062106 (2019)
Keywords: Machine Learning, Square Ice, Loop Algorithm
We present a deep reinforcement learning framework where a machine agent is trained to search for a policy to generate a ground state for the square ice model by exploring the physical environment. After training, the agent is capable of proposing a sequence of local moves to achieve the goal. Analysis of the trained policy and the state value function indicates that the ice rule and loop-closing condition are learned without prior knowledge. We test the trained policy as a sampler in the Markov chain Monte Carlo and benchmark against the baseline loop algorithm. This framework can be generalized to other models with topological constraints where generation of constraint-preserving states is difficult.
Wen-Han Kao, Peter Holdsworth, and Ying-Jer Kao
Phys. Rev. B 93, 180410(R) (2016)
Keywords: Dipolar Spin Ice, Monte Carlo, Neutron Scattering
We present numerical studies of dipolar spin ice in the presence of a magnetic field slightly tilted away from the [111] axis. We find a first-order transition from a kagome ice to a q = X state when the external field is tilted toward the [11-2] direction. This is consistent with the anomalous critical scattering previously observed in the neutron scattering experiment on the spin ice material Ho2Ti2O7 in a tilted field [T. Fennell et al., Nat. Phys. 3, 566 (2007)]. We show that this ordering originates from the antiferromagnetic alignment of spin chains on the kagome planes. Our result captures the features observed in the experiments and points to the importance of the dipolar interaction in determining ordered states in the spin ice materials.
Vacancy spectroscopy of non-Abelian Kitaev spin liquids, Quantum Materials for Emergent Applications in Quantum Science Workshop, Telluride, CO, USA (2024) [Invited]
Vacancy spectroscopy of non-Abelian Kitaev spin liquids, APS March Meeting, Minneapolis, MN, USA (2024)
Disorder in the Kitaev Spin Liquid, Department of Physics, University of Wisconsin Madison, Madison, WI, USA (2023)
Spin- and Flux-gap Renormalization in the Random Kitaev Spin Ladder, Blackboard Seminar, Department of Physics, Technical University of Munich, Munich, Germany (2023)
Spin- and Flux-gap Renormalization in the Random Kitaev Spin Ladder, CompQu Seminar of National Center for Theoretical Sciences Physics Division, Taiwan, online (2022)
Flux-gap Renormalization in the Random Kitaev Spin Ladder, APS March Meeting, Chicago, IL, USA (2022) talk video
Vacancy-induced Low-energy Density of States in the Kitaev Spin Liquid, Condensed Matter Physics in the City (CMPC2021), online (2021) talk video
SDRG Study of Random Kitaev Chains and Ladders, APS March Meeting, online (2021)
Vacancy-induced Low-energy Density of States in the Kitaev Spin Liquid, waiting for the conference on Highly Frustrated Magnetism (wHFM21), online (2021)
Stability and Fluctuation of Snake-like Magnetic Domain in Kagome Spin Ice, Annual Meeting of the Physical Society of Taiwan (TPS), Taipei, Taiwan (2018)
Field-induced Ordering in Dipolar Spin Ice, Awarding talk for best paper award, NTU Center for Theoretical Physics, Taipei, Taiwan (2017) talk video (Mandarin)
Field-induced Ordering in Dipolar Spin Ice, 8th International Conference on Highly Frustrated Magnetism (HFM), Taipei, Taiwan (2016)
Spin- and Flux-gap Renormalization in the Random Kitaev Spin Ladder, Quantum Localization and Glassy Physics Summer School (QLGP), Cargèse, France (2023)
Spin- and Flux-gap Renormalization in the Random Kitaev Spin Ladder, 11th International Conference on Highly Frustrated Magnetism (HFM), Paris, France (2022)
Stability and Fluctuation of Snake-like Magnetic Domains in Kagome Spin Ice, Advances in Strongly Correlated Electronic Systems (ASCES2019), Minneapolis, MN, USA (2019)
Learning to Discover Loop Algorithm on Spin Ice Model, 21th International Conference on Magnetism (ICM), San Francisco, CA, USA (2018)
Stability and Fluctuation of Snake-like Magnetic Domains in Kagome Spin Ice, 9th International Conference on Highly Frustrated Magnetism (HFM), Davis, CA, USA (2018)
Emergent Snake-like Magnetic Domains in Canted Kagome Spin Ice, NCTS Workshop on Correlated Quantum Many-body Systems, Hsinchu, Taiwan (2018)
Field-induced Phase Transitions of Dipolar Spin Ice Under [111] Magnetic Field, Annual Meeting of the Physical Society of Taiwan (TPS), Hsinchu, Taiwan (2015)