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Thermo-osmosis is a nanoscale fluid flow along solid surfaces driven by temperature variation. In this paper, a model for thermo-osmosis is proposed within a slip-flow theory for molecular fluids. The key is to combine the generalized slip-flow theory for molecular gases with the effects of fluid–solid interaction potentials. By tuning the potentials, or molecular “affinity,” the theory reproduces the reversal of flow direction observed in molecular simulations: when the fluid–solid interaction is favorable (unfavorable), the flow is directed toward the hot (cold) region. This work provides a starting point toward a universal model of slip phenomena in gases and liquids at the nanoscale.
Tsuji, et al, Phys. Rev. Fluids (2025) link
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Mapping the Thermal Forces That Push Particles through Liquids
Thermo-osmotic slip flows around microparticles: (left) COOH-mod (right) NH2-mod. Heating initiated at t = 0 sec. Tsuji, et al., Phys. Rev. Appl. (2023)
Press release from Kyoto University & JST
Tsuji, et al, Phys. Rev. Appl. (2023)
Elaborating micro- and nanoscale heat using lasers is an emerging experimental technique to induce fluid flows and to control nanomaterial motions; this paper provides a theoretical tool to explore them. When focused lasers are irradiated to microfluidic systems, we can heat up, selectively and locally, fluids and/or solid-fluid interfaces such as thin-metal films. This localized heat generates various thermally-induced transport of fluids and dispersed objects. Considering that flow computation requires a decent amount of training cost, the easy-access instant analytical tool developed here is helpful for researchers without a fluid-mechanics background to explore complex phenomena in their own fields.
Tsuji, et al, Phys. Rev. Fluids (2024) link
Thermophoretic separation of colloid mixture: Selective trapping of PS beads
Tsuji, et al, Phys. Rev. Appl. (2018)
Hydrodynamic inter-particle interaction accelerates the orbital speed of particles under the irradiation of an optical vortex Tsuji, et al, Nanoscale (2020)
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Setoura, Tsuji, et al.,
Nanoscale (2019)
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Tsuji, et al., Nanoscale (2020)
Flow induced by a discontinuous boundary temperature.
Taguchi & Tsuji, J. Fluid. Mech. (2020)
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The impulsive swirl of a gas
Flow induced by impulsive rotation of a sphere.
Taguchi, Tsuji & Kotera, J. Fluid. Mech. (2021)
Thermophoresis of colloids in a micro-gap Soret cell; sign inversion for different solvent
Tsuji, et al., Micro Nano Lett. (2017)
Laser-induced thermophoresis at the inlet of a microchannel constriction
Tsuji, et al., Phys. Rev. Appl (2018)
Orbital motion of a particle driven by
an optical vortex in a microscale
double orifice
Nakajima, et al., Sci. Rep. (2021)
Velocity distribution functions near a solid oscillating boundary
Tsuji and Aoki, J. Comput. Phys. (2013)
Switching between laser-induced thermal-convection-accumulation mode (left) and thermophoretic-depletion mode (right) Tsuji, et al, Electrophoresis (2021)
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Tsuji, et al., Electrophoresis (2021)