The real world is seamlessly merging with the cyber world. In this transition, advanced carbon materials and sensor technologies play a critical role by translating complex physical and chemical information into actionable electronic data. Powered by this data and artificial intelligence (AI), we are predicting future trends and creating new value for society. By harnessing the unique optoelectronic properties of the nanocarbon materials, we establish highly intelligent analytical platforms. Our core expertise lies in the carbon-molecular interface, where we precisely engineer quantum defects and surface chemistry. Moving beyond empirical molecular recognition, we employ rational inverse design and AI to program how carbon lattices interact with diverse target molecules. There is significant motivation to extend these rationally designed interfaces to real-world, multiscale engineering applications. By bridging atomic-level quantum control with robust material integration, our intelligent carbon systems are expanding from precision digital healthcare to broader industrial applications. These platforms are innovating the future of chemical, biological, and materials engineering.