Ground state of antiferromagnetic NiO obtained from multiscale modeling
Multiscale Modelling in Magnets:
The magnetization dynamics are described by the traditional Landau-Lifshitz-Gilbert (LLG) equation that consists of the precession of magnetic moment around an effective field and dissipation of energy in terms of Gilbert damping. To model the magnetization dynamics the LLG equation is solved with the effective field that is already present in a system. The effective field is calculated from the total ground state energy of a magnetic system. Such energy includes magnetic exchange, anisotropy, and other types of energy contributions that can be calculated within a density functional theory (DFT) approach. The multiscale modeling in magnets provides important ground state characteristics.
Reference: Schmidt, Mondal et. al. Phys. Rev. B 102, 214436 (2020)
Antiferromagnetic spintronics:
Antiferromagnets consist of two opposite spins with equal magnitude. The exchange energies between these two spins are very strong. The antiferromagnets show faster dynamics than ferromagnets due to their natural THz resonance frequency. The antiferromagnets are abundant in the world and they do not possess any stray fields. Owing to these fundamental properties, the antiferromagnetic spins can be densely packed in a small magnetic domain and they are robust against external perturbation which makes antiferromagnets a perfect material for data storage devices. The switching of antiferromagnets shows 90 degrees that cost less energy than 180 degrees switching.
Ref: Mondal et. al. Phys. Rev. B 100, 060409 (2019)
Antiferromagnetic spin manipulation in CuMnAs
A typical demagnetization curve under the influence of laser heating in Nickel
Ultrafast Spin Dynamics:
The pioneering work of femsotsecond control of magnetism in Ni was discovered in 1996 which showed the spins can be manipulated at ultrafast timescales. Such remarkable achievement has changed the technological solutions of data storage devices. Not only the ultrafast demagnetization, but also, the thermal switching in ferrimagnets can be explained by the solutions of the LLG equations having two sublattices with the laser heating included. Apart from the traditional LLG spin torques, there could be several other spin torques e.g., spin-transfer torque, spin-orbit torque, optical spin-orbit torque, and others contributing to the LLG spin dynamics. The effects of these torques need to be investigated for several classes of magnets.
Reference: Mondal et. al. Phys. Rev. B 98, 214429 (2018)
Terahertz nutation resonance:
Under the influence of external drive, the ferromagnetic spins can resonantly be driven at GHz frequencies - typically known as ferromagnetic resonance (FMR). The consequent switching of spins is limited by nanosecond timescale which is determined by the inverse of GHz frequency. A completely different mechanism of spin nutation dictates that the ferromagnets can even be manipulated resonantly at higher frequency e.g., at THz. The appearance of THz resonant frequency means that the ferromagnetic spins can now be manipulated at picosecond timescales. A lot of opportunities can be explored in this nutation dynamics not only in ferromagnets but also in antiferromagnets and non-collinear magnetic structures.
Ref: Mondal et. al. Phys. Rev. B 103, 104404 (2021)
Mondal et. al. JMMM 579, 170830 (2023)
The nutation dynamics occur at femtosecond timescales
Relativistic theory of electron spin:
Spin, in quantum mechanics, is an intrinsic property of an elemental particle e.g., the electron and the electron's spin can only be introduced within the relativistic Dirac theory. However, in contrast to nonrelativistic quantum mechanics, the definition of the spin operator is not unique in relativistic quantum mechanics. In nonrelativistic quantum mechanics, the spin is expressed by the Pauli spin matrices. On contrary, in a relativistic formulation, the spin angular momentum cannot be defined separately because the total angular momentum has to be conserved. Therefore, the definition of spin angular momentum depends on the definition of the orbital angular momentum.
Reference: Mondal et al. J. Phys: Condens. Matter 32, 455802 (2020)
Research Funding
2024 - 2025: Paired Early Career Fellowship in Applied Research (PECFAR) award by Indo-German Science and Technology Centre (IGSTC).
2024 - 2026: Startup Research Grant (SRG) from the Department of Science and Technology (DST) Science & Engineering Research Board (SERB).
2023-2026: Faculty Research Scheme (FRS) from IIT (ISM) Dhanbad.
2020 - 2022: VR international postdoc grant from the Swedish Research Council (Vetenskapsrådet), Sweden.
2019 - 2020: Alexander von Humboldt postdoctoral grant from the Alexander von Humboldt foundation. Germany
2019 - 2019: Zukunftskolleg Mentorship grant from the Universität Konstanz, Germany