Researcher at Istituto dei Sisitemi Complessi- Consiglio Nazionale delle Ricerche
Dipartimento Di Fisica- Università di Roma La Sapienza
Piazzale Aldo Moro 5, 00185-Rome, Italy
Fermi Building - Room 410
Phone: 0039649913480
Interests: Microlasers, Random photonics, Biosensing, Nonlinear Optics
Highlights:
For the first time we report the ultrametric structure of the replica space with clustered domains in random lasers, as predicted in the Parisi Ansatz.
In the ultrametric space all triangles are either equilateral or isosceles with the third side shorter than the two equal ones. This is the topology of hierarchic structures and it is intrinsic of spin glasses.
We give the experimental prove of this universal behaviour in photonics by showing that the number of the states forming isosceles triangles in the metric space increases through the laser threshold giving rise to the construction of a genealogical tree.
Moreover, from the hierarchical topology of the states we obtain a direct observation of the complex energy landscape with evident breaking of ergodicity in the glassy regime.
The number of states forming isosceles triangle increases with input energy. There is a transition from flat to hierarchical topology at spin glass transition.
We successfully use polymeric whispering gallery microlasers as biosensors for detecting small amounts of proteins, down to 400 pg. They have the advantage of working in free space without any need for waveguiding for input excitation or output signal detection. The photonic microsensors can be easily patterned on microscope slides and operate in air and solution. We estimate the limit of detection up to 148 nm/RIU for three different protein dispersions. In addition, the sensing ability of passive spherical resonators in the presence of dielectric nanoparticles that mimic proteins is described by massive ab initio numerical simulations.
We highlight the impressing experiments by Tivedi et al. on thermally reconfigurable random lasers. Janus micro-colloids act as heat reservoirs and attract titania particles due to the Soret effect. Thanks to their accumulation around patterns of "hot colloids" and under pumping programmable random laser action is nicely demonstated.
We realize flexible smart photonic labels made of doped liquid droplets encapsulated in polymeric matrix. The innovative hybrid whispering gallery and random lasing emission offers a multitude of spectroscopic encoding schemes for the realization of photonic barcodes and labels to be employed in anticounterfeiting applications and multiplexed bioassays.
Statistical mechanics analysis of fluorescence imaging provides new insights into the complex entrapment of light in disordered heterostructures. Heterogeneous random lasers made of ribbon-like and highly porous fibers show laser action from separated micrometric domains that alternatively switch on and off by tuning the pumping light intensity.
We demonstrate that the configuration of random laser lines is uniquely dependent on the structure of porous materials at micrometric scale. Differently from other spectroscopic techniques that provide mainly and accurately the chemical composition, RL spectra can be used to identify the micro- scopic structure and the aggregation state of the compounds.