本實驗室將推廣量子磁性材料的基礎及應用及推廣量子磁性材料的關鍵技術-中子散射技術,中子散射技術解析量子磁性材料中磁結構和自旋動力學的唯一工具,我們的團隊已經在該領域取得了突出的進展及成果。
Magnetic structure analysis (磁結構分析)
我們將考慮材料中的結構及磁的對稱性以釐清磁電耦合及壓電耦合相關的物理機制
我們專門使用中子單晶繞射偵測微弱磁結構的信號以解決粉末繞射其解析度不足而導致無法判斷磁結構的窘境
T. W. Kuo* et al., “Enhanced Néel-type skyrmion stability in polar VOSe2O5 through tunable magnetic anisotropy under pressure”, Phys. Rev. B (2025)
We recently uncovered two distinct magnetic structures in polar VOSe2O5 using powder neutron diffraction: a commensurate three-up–one-down ferrimagnetic order at low temperature (1.8 K) and an incommensurate cycloidal spin structure at 6 K. These findings reveal the presence of strong magnetic anisotropy in the system. By applying hydrostatic pressure, we successfully tuned this anisotropy—enhancing the stability of the Néel-type skyrmion phase. Under 14.2 kbar, the skyrmion zone expands nearly threefold in the magnetic field–temperature phase diagram. This work demonstrates how magnetic anisotropy can be engineered to control topological spin textures, offering new routes toward skyrmion-based spintronic applications.
H. C. Wu* et al., “Observation of thermally induced piezomagnetic switching in Cu2OSeO3 polymorph synthesized under high-pressure”, Advanced Physics Research 3, 2400054 (2024)
We report the first observation of a finite enhancement of the weak ferromagnetic component in the Cu-based compound under uniaxial stress, providing evidence of the piezomagnetic effect and confirming the magnetic space group determination resolved by neutron diffraction. An intriguing sign change in the piezomagnetic coefficient holds the potential for realizing new functionality in switchable magnetic domains by manipulating pressure.
H. C. Wu*, A. Nakamura, D. Okuyama, K. Nawa, D. Aoki, and T. J. Sato, “Unraveling the magnetic structure of YbNiSn single crystal via crystal growth and neutron diffraction”, J. Magn. Magn. Mater. 584, 171054 (2023)
Neutron and x-ray diffraction experiments were performed on the ternary intermetallic compound YbNiSn, formerly categorized as a ferromagnetic Kondo compound. The proposed magnetic structures at zero field and 1 T correspond to the magnetic space groups of Pn'm'a and Pnm'a', respectively. The piezomagnetic effect and the switch between the two magnetic space groups by the external stress, which could be detected by the anomalous Hall effect, are proposed.
C. Chaffey, H. C. Wu*, H. Jin, P. Sherpa, P. Klavins, M. Avdeev, S. Aji, R. Shimodate, K. Nawa, T. J. Sato, V. Taufour, and N. J. Curro, “Magnetic structure and Kondo lattice behavior in CeVGe3: an NMR and neutron scattering study”, Phys. Rev. B 108, 115163 (2023)
We present neutron diffraction measurements on a single crystal and powder of CeVGe3. This material exhibits heavy fermion behavior at low temperatures, accompanied by antiferromagnetic (AFM) order below 5.8 K. We find that the magnetic structure is incommensurate with AFM helical structure, characterized by a magnetic modulated propagation vector of (0, 0, 0.49) with in-plane moments rotating around the 𝑐 axis.