Transition metal dichalcogenides (TMDs, MX2 with M = Mo, W and X = S, Se) are a new class of two-dimensional (2D) semiconductors. We fabricate atomically thin samples, create heterostructures and devices, and employ optical and electrical probes to study their unique properties. Recent topics of interests include valley- and spin-dependent transport, exciton condensation and strong correlation physics of moire flat bands.
Reviews
Photonics and optoelectronics of two-dimensional semiconductor transition metal dichalcogenides
K. F. Mak and J. Shan, Nature Photon. 10, 216-226 (2016).
Light-valley interactions in 2D semiconductors
K. F. Mak, D. Xiao, and J. Shan, Nature Photon. 12, 451-460 (2018).
Opportunities and challenges of interlayer exciton control and manipulation
K. F. Mak and J. Shan, Nature Nanotech. 13, 974-976 (2018).
Optical properties of TMDs
Atomically thin MoS2: A new direct-gap semiconductor
K. F. Mak, Changgu Lee, J. Hone, J. Shan, and T. F. Heinz, Phys. Rev. Lett. 105, 136805 (2010).
K. He, K. F. Mak, C. Pools, and J. Shan, Nano Lett. 13, 2931–2936 (2013).
Valley degeneracy breaking by magnetic field in monolayer MoSe2
D. MacNeill, C. Heikes, K. F. Mak, Z. Anderson, A. Kormányos, V. Zólyomi, J. Park, and D. C. Ralph, Phys. Rev. Lett. 114, 037401 (2015).
Valley- and spin-polarized Landau levels in monolayer WSe2
Z. Wang, J. Shan, and K. F. Mak, Nature Nanotech. 12, 144–149 (2017).
Valley dependent physics
Control of valley polarization in monolayer MoS2 by optical helicity
K. F. Mak, K. He, J. Shan, and T.F. Heinz, Nature Nanotech. 7, 494–498 (2012).
The valley Hall effect in MoS2 transistors
K. F. Mak, K. L. McGill, J. Park, and P. L. McEuen, Science 344, 1489-1492 (2014).
Valley- and spin-polarized Landau levels in monolayer WSe2
Z. Wang, J. Shan, and K. F. Mak, Nature Nanotech. doi:10.1038/nnano.2016.213 (2016).
Electrical control of the valley Hall effect in bilayer MoS2 transistors
J. Lee, K. F. Mak, and J. Shan, Nature Nanotech. 11, 421-425 (2016).
Valley magnetoelectricity in single-layer MoS2
J. Lee, Z. Wang, H. Xie, K. F. Mak, and J. Shan, Nature Mater. 16, 887-891 (2017).
Strongly interaction-enhanced valley magnetic response in monolayer WSe2
Z. Wang, K. F. Mak, and J. Shan, Phys. Rev. Lett. 120, 066402 (2018)
Excitonic effects in TMDs
Tightly bound trions in monolayer MoS2
K. F. Mak, Keliang He, Changgu Lee, Gwan Hyoung Lee, J. Hone, T.F. Heinz, and J. Shan, Nature Mater. 12, 207–211 (2013).
Orientation of luminescent excitons in layered nanomaterials
J. A. Schuller, S. Karaveli, T. Schiros, K. He, S. Yang, I. Kymissis, J. Shan, and R. Zia, Nature Nanotech. 8, 271–276 (2013).
Tightly bound excitons in monolayer WSe2
K. He, N. Kumar, L. Zhao, Z. Wang, K.F. Mak, H. Zhao, and J. Shan, Phys. Rev. Lett. 113, 026803 (2014).
Electrical tuning of interlayer exciton gases in WSe2 bilayers
Z. Wang, Y.-H. Chiu, K. Honz, K. F. Mak, and J. Shan, Nano Lett. 18, 137-143 (2018).
Ultrafast and nonlinear optical properties of TMDs
Observation of intense second harmonic generation from MoS2 atomic crystals
L. M. Malard, T. V. Alencar, A.P.M. Barboza, K. F. Mak, and A.M. de Paula, Phys. Rev. B 87, 201401 (2013).
Probing symmetry properties of few-layer MoS2 and h-BN by optical second-harmonic generation
Y. Li, Y. Rao, K. F. Mak, Y. You, S. Wang, C. R. Dean, and T. F. Heinz, Nano Lett. 13, 3329-3333 (2013).
Controlling the spontaneous emission rate of monolayer MoS2 in a photonic crystal nanocavity
X. Gan, Y. Gao, K. F. Mak, X. Yao, R. J. Shiue, A. van der Zande, M. Trusheim, F. Hatami, T. F. Heinz, J. Hone, and D. Englund, Appl. Phys. Lett. 103, 181119 (2013).
P. Dey, J. Paul, Z. Wang, C. E. Stevens, C. Liu, A. H. Romero, J. Shan, D. J. Hilton, and D. Karaiskaj, Phys. Rev. Lett. 116, 127402 (2016).