Simulate strong light propagation in 3D materials based on nonlinear Schrödinger equation, including
Beam diffraction
Self-focusing (Kerr nonlinearity) and self-defocusing (plasma effect)
Photoionization and avalanche ionization
Free-carrier absorption
Simulate ablation of 3D materials (fused silica, quartz, sapphire, and PMMA)
Simulate ablation of 2D transition metal dichalcogenides (MoS2, WS2, and WSe2)
Analyze etalon effect in 2D or quasi-2D materials.
Develop Keldysh’s photoionization theory for 2D systems.
Develop modified multiple-rate equations for VB (valance band)-CB (conduction band)-XA (exciton state) systems.
Develop modified two-temperature model for 2D systems.
In 2017-2018, we can Prof. Tsing-Hua Her (University of North Carolina at Charlotte, USA) cooperated with multiple prestigious scholars of Air Force Research Laboratory in USA to investigate photoelectron emission from 1D carbon nanotubes. By the aid of strong exciton resonances and high damage threshold of 1D carbon nanotube, ultra-bright and ultrafast photoemission can be realized. This work has been published in the high-impact journal: “Nano Letters” (Nano Lett. 19, 158-164 (2018)).
Since one of the major expertise of Prof. Tsing-Hua Her is in the laser ablation and micromachining of 3D bulk materials, during 2018-2022, we extended from that field to investigate the strong-field physics of 2D materials, such as the most popular 2D material: graphene and a variety of transition metal dichalcogenides TMDs (MoS2, WS2, MoSe2, and WSe2). This work is an international multi-cooperation project. 2D TMD samples were supplied by Prof. Wen-Hao Chang (National Yang Ming Chao Tung University, NYCU, in Taiwan), while parts of 800-nm laser-ablation experiments with variable pulse durations were proceeded by Prof. Chih-Wei Lou (NYCU). We discovered that several mechanisms play the important roles in the optical dielectric breakdown of 2D materials. Firstly, instead of complicated wave propagation in 3D materials (accompanied with the effects listed above) that is required nonlinear Schrödinger equation for description, the field in 2D materials becomes quasi-static because of strong etalon effect. Several our experimental results regarding this issue have been published in “AIP Advances” (AIP Adv. 12, 015217 (2022)) and “Scientific Reports” (Sci. Rep. 12, 1-9 (2022)). Secondly, many nonlinear optical processes, such as multiphoton and tunneling ionization, plasma heating, and the subsequent avalanche ionization in 2D materials change significantly from their counterparts in 3D cases. It is because of the change of dimensionality (3D→2D) and the significant exciton effect under strong quantum confinement. Therefore, several necessary modifications on the existed theoretical models for 3D materials are required. Prof. Her and I have completed parts of preliminary works and we will devoted to comparing the theoretical predictions and experimental results in the following several years.