Carbon Adsorbents for Medicine and Environmental Protection
National Aviation University, Kyiv, Ukraine
Professor
Alexander M. Puziy
E-mail: alexander.puziy at gmail.com
Research Interests
Development of novel adsorbents (carbonaceous, biomass, inorganic or composite) for medical applications (enterosorbents, hemoadsorbents, food or fodder additives)
Development of nanostructured carbon adsorbents with enhanced performance for adsorption, catalysis and energy storage
Functionalization of carbon materials by heteroatoms (oxygen, nitrogen, phosphorus)
Development of biomass-based adsorbents
Development of carbon adsorbents from biomass, agricultural waste materials and hard coal
Adsorption of biomolecules, organic pollutants and heavy metals
Achievements
Medicinal sorption materials: Hemoadsorbents (SCN, SCS, KAU, SCN-D, SCNo-KMg), Enterosorbents (SCN, Carbovit, Ultrasorb, Pectopal, Carboxikam, Carbodon)
Fodder additive (activated carbon and agricultural wastes) capable of adsorbing a wide range of toxins (aflotoxins, psticides, heavy metals, radionuclides)
Functionalization of carbonaceous materials with phosphorus-containing groups
Phosphorus-enriched carbons for double layer supercapacitors
Technology for processing of hard coal (anthracite) into carbon adsorbent
Technology for processing of PET (polyethileneterephtalate) into carbon adsorbent
Technology for processing of biomass wastes into carbon adsorbent
Scientific Cooperation
Maria Skłodowska-Curie University, Lublin (Poland)
Instituto de Ciencia y Technologia del Carbono (INCAR), Oviedo (Spain)
The Royal Institute of Technology (KTH), Stockholm (Sweden)
Royal Military Academy, Brussels (Belgium)
The University of Queensland, Brisbane (Australia)
Institute of Catalysis, Krakow (Poland)
Nicolaus Copernicus University, Torun (Poland)
University of Brighton, Brighton (UK)
Institute of Nonclassic Chemistry, Leipzig (Germany)
University of Alicante, Alicante (Spain)
University of South Carolina, Columbia (USA)
Institute of Chemistry, Chisinau (Moldova)
Main Publications
[1] A.M. Puziy, P. Lodewyckx, J.A. Ritter, A.D. Ebner, F. Suarez-Garcia, Editorial: Physisorption of Gases: Adsorbent Characterization, Adsorbent-Adsorbate Equilibrium and Kinetics, Front. Chem. 9 (2021) 668553. https://doi.org/10.3389/fchem.2021.668553.
[2] N.I. Ermokhina, V. V. Shvalagin, N.I. Romanovska, P.A. Manoryk, R.Y. Barakov, M.O. Kompanets, V.I. Sapsay, D.O. Klymchuk, A.M. Puziy, Synthesis and characterization of different binary and ternary phase mixtures of mesoporous nanocrystalline titanium dioxide, SN Appl. Sci. 3 (2021) 491. https://doi.org/10.1007/s42452-021-04474-y.
[3] V. Sydorchuk, O.I. Poddubnaya, M.M. Tsyba, O. Zakutevskyy, O. Khyzhun, S. Khalameida, A.M. Puziy, Photocatalytic degradation of dyes using phosphorus-containing activated carbons, Appl. Surf. Sci. 535 (2021) 147667. https://doi.org/10.1016/j.apsusc.2020.147667.
[4] A.M. Puziy, O.I. Poddubnaya, B. Gawdzik, J.M.D. Tascón, Phosphorus-containing carbons: Preparation, properties and utilization, Carbon. 157 (2020) 796–846. https://doi.org/10.1016/j.carbon.2019.10.018.
[5] V. Shvalagin, N. Ermokhina, N. Romanovska, R. Barakov, P. Manorik, V. Sapsay, S. Shcherbakov, O. Poddubnaya, A. Puziy, Mesoporous TiO2 microspheres with improved efficiency for photooxidation of volatile organic compounds, Res. Chem. Intermed. 45 (2019) 4133–4148. https://doi.org/10.1007/s11164-019-03896-z.
[6] V. Sydorchuk, O.I. Poddubnaya, M.M. Tsyba, O. Zakutevskyy, O. Khyzhun, S. Khalameida, A.M. Puziy, Activated carbons with adsorbed cations as photocatalysts for pollutants degradation in aqueous medium, Adsorption. 25 (2019) 267–278. https://doi.org/10.1007/s10450-018-00006-0.
[7] N.I. Ermokhina, V. V. Shvalagin, N.I. Romanovska, N.A. Sydorova, P.A. Manoryk, R.Y. Barakov, M.M. Shcherbatyuk, D.O. Klymchuk, A.M. Puziy, Photocatalytic Activity of Mesoporous Titanium Dioxide Stabilized with Lanthanum in the Gas-Phase Oxidation of Ethanol, Theor. Exp. Chem. 53 (2018) 395–401. https://doi.org/10.1007/s11237-018-9537-y.
[8] Л. Борко, Н.В. Власенко, Ж. Коппань, А. Бекк, А.М. Пузий, Влияние редокс- и кислотных свойств нанофазных катализаторов Ga-H-ZSM-5, модифицированных переходными металлами, на восстановление закиси азота метаном, Теоретическая и Экспериментальная Химия. 54 (2018) 227–234.
[9] L. Borkó, N. V. Vlasenko, Z. Koppány, A. Beck, A.M. Puziy, Effect of Redox and Acid Properties of Ga–H-ZSM-5 Nanophase Catalysts Modified by Transition Metals on the Reduction of Nitrous Oxide by Methane, Theor. Exp. Chem. 54 (2018) 247–254. https://doi.org/10.1007/s11237-018-9570-x.
[10] A.M. Puziy, O.I. Poddubnaya, O. Sevastyanova, Carbon materials from technical lignins: recent advances, Top. Curr. Chem. 376 (2018) 33. https://doi.org/10.1007/s41061-018-0210-7.
[11] C. Huang, A.M. Puziy, O.I. Poddubnaya, D. Hulicova-Jurcakova, M. Sobiesiak, B. Gawdzik, Phosphorus, nitrogen and oxygen co-doped polymer-based core-shell carbon sphere for high-performance hybrid supercapacitors, Electrochim. Acta. 270 (2018) 339–351. https://doi.org/10.1016/j.electacta.2018.02.115.
[12] A.M. Puziy, O.I. Poddubnaya, M. Sobiesiak, B. Gawdzik, Assessment of the structural evolution of polyimide-derived carbons obtained by phosphoric acid activation using Fourier transform infrared and Raman spectroscopy, Adsorpt. Sci. Technol. 35 (2017) 403–412. https://doi.org/10.1177/0263617417693627.
[13] O.L. Stroyuk, N.I. Ermokhina, G. V. Korzhak, N.S. Andryushina, V. V. Shvalagin, A. V. Kozytskiy, P.A. Manoryk, R.Y. Barakov, S.Y. Kuchmiy, M. Shcherbatyuk, V.I. Sapsay, A.M. Puziy, Photocatalytic and photoelectrochemical properties of hierarchical mesoporous TiO2 microspheres produced using a crown template, J. Photochem. Photobiol. A Chem. 334 (2017) 26–35. https://doi.org/10.1016/j.jphotochem.2016.10.039.
[14] N. V. Vlasenko, Y.N. Kochkin, A.M. Puziy, P.E. Strizhak, Crucial Role of Weak Acid Sites for Catalytic Performance of Zeolites in Ethyl tert-butyl Ether Synthesis, Chem. Eng. Commun. 204 (2017) 937–941. https://doi.org/10.1080/00986445.2017.1328411.
[15] V.V. Sydorchuk, S.V. Khalameida, O.I. Poddubnaya, M.M. Tsyba, A.M. Puziy, Cation-containing active carbons as photocatalysts for dyes degradation, Him. Fiz. Ta Tehnol. Poverhni. 8 (2017) 422–431. https://doi.org/10.15407/hftp08.04.422.
[16] Н.И. Ермохина, В.В. Швалагин, Н.И. Романовская, Н.А. Сидорова, П.А. Манорик, Р.Ю. Бараков, Н.Н. Щербатюк, Д.А. Климчук, А.М. Пузий, Фотокаталитическая активность мезопористого диоксида титана, стабилизированного лантаном, в процессе газофазного окисления этанола, Теоретическая и Экспериментальная Химия. 53 (2017) 368–374. https://www.elibrary.ru/item.asp?id=30797042.
[17] A.M. Puziy, Y.N. Kochkin, O.I. Poddubnaya, M.M. Tsyba, Ethyl tert-butyl ether synthesis using carbon catalysts from lignocellulose, Adsorpt. Sci. Technol. 35 (2017) 473–481. https://doi.org/10.1177/0263617417696091.
[18] Y.N. Kochkin, N. V. Vlasenko, V.L. Struzhko, A.M. Puziy, P.E. Strizhak, Methanol carboxylation over zirconium dioxide: Effect of catalyst phase composition on its acid-base spectrum and direction of catalytic transformations, Can. J. Chem. Eng. 94 (2016) 745–751. https://doi.org/10.1002/cjce.22435.
[19] С.І. Трофименко, Н.В. Сич, М.М. Циба, О.І. Піддубна, О.М. Пузій, Вуглецеві адсорбенти з кукурудзяних качанів, що одержані мікрохвильовим активуванням фосфорною кислотою, Вісник Прикарпатського Національного Університету Імені Василя Стефаника. Серія Хімія. 20 (2016) 67–71.
[20] A.M. Puziy, O.I. Poddubnaya, A. Derylo-Marczewska, A.W. Marczewski, M. Blachnio, M.M. Tsyba, V.I. Sapsay, D.O. Klymchuk, Kinetics of protein adsorption by nanoporous carbons with different pore size, Adsorption. 22 (2016) 541–552. https://doi.org/10.1007/s10450-015-9723-3.
[21] A.M. Puziy, O.I. Poddubnaya, B. Gawdzik, M. Sobiesiak, Comparison of heterogeneous pore models QSDFT and 2D-NLDFT and computer programs ASiQwin and SAIEUS for calculation of pore size distribution, Adsorption. 22 (2016) 459–464. https://doi.org/10.1007/s10450-015-9704-6.
[22] A.L. Stroyuk, N.I. Ermokhina, A.V. Korzhak, N.S. Andryushina, A. V. Kozytskiy, P.A. Manorik, V.G. Ilyin, A.M. Puziy, V.I. Sapsai, N.N. Shcherbatyuk, Photocatalytic and Photoelectrochemical Characteristics of Mesoporous Titanium Dioxide Microspheres, Theor. Exp. Chem. 51 (2015) 183–190. https://doi.org/10.1007/s11237-015-9414-x.
[23] А.Л. Строюк, Н.И. Ермохина, А.В. Коржак, Н.С. Андрюшина, А.В. Козицкий, П.А. Манорик, В.Г. Ильин, А.М. Пузий, В.И. Сапсай, Н.Н. Щербатюк, Фотокаталитические и фотоэлектрохимические свойства мезопористых микросфер диоксида титана, Теоретическая и Экспериментальная Химия. 51 (2015) 176–184.
[24] Н. Чикун, Б. Пасальський, О. Пузій, Ефективність вітчизняних адсорбентів при очищенні води від йонів Феруму (ІІІ), Товари і Ринки. (2015) 170–175.
[25] Д. Кисельов, В. Овчинніков, В. Амірханов, С. Ставицька, М. Циба, О. Піддубна, О. Пузій, Модифікування активованого вугілля карбациламідофосфатом для сорбції йонів Cu(ІІ) та La(ІІІ), Вісник Київського Національного Університету Імені Тараса Шевченка. 50 (2014) 38–41.
[26] С.І. Трофименко, Н.В. Сич, О.М. Пузій, Н.Ю. Чикун, Б.К. Пасальський, Застосування модифікованих вуглецевих сорбентів для очистки питної води, Інтегроване Управління Водними Ресурсами. (2014) 277–281.
[27] M. Myglovets, O.I. Poddubnaya, O. Sevastyanova, M.E. Lindström, B. Gawdzik, M. Sobiesiak, M.M. Tsyba, V.I. Sapsay, D.O. Klymchuk, A.M. Puziy, Preparation of carbon adsorbents from lignosulfonate by phosphoric acid activation for the adsorption of metal ions, Carbon. 80 (2014) 771–783. https://doi.org/10.1016/j.carbon.2014.09.032.
[28] A.M. Puziy, J.M.D. Tascón, Reseña Histórica: Acerca de la Regla de Gurvitsch, Mater. En Adsorción y Catálisis. (2014) 59–62. http://www.adsorcion.com/uploads/revistas/MAyC_num_7-SIETE_ SEPT 2014.pdf.
[29] S.S. Stavitskaya, O.I. Poddubnaya, N.N. Tsyba, A.M. Puziy, Catalytic Properties of Phosphorus-Containing Charcoals in Ethyl Acetate Hydrolysis, Theor. Exp. Chem. 50 (2014) 187–190. https://doi.org/10.1007/s11237-014-9364-8.
[30] О. Пузій, Б. Пасальський, Н. Чикун, Фосфоровмісні вуглецеві сорбенти для очистки води, Товари і Ринки. 17 (2014) 159–166.
[31] C. Huang, A.M. Puziy, T. Sun, O.I. Poddubnaya, F. Suárez-García, J.M.D. Tascón, D. Hulicova-Jurcakova, Capacitive Behaviours of Phosphorus-Rich Carbons Derived from Lignocelluloses, Electrochim. Acta. 137 (2014) 219–227. https://doi.org/10.1016/j.electacta.2014.05.101.
[32] S.S. Stavitskaya, V.M. Vikarchuk, M.F. Kovtun, O.I. Poddubnaya, A.M. Puziy, Adsorption of copper ions by carbon adsorbents modified by phosphoric acid at different temperatures, J. Water Chem. Technol. 36 (2014) 110–114. https://doi.org/10.3103/S1063455X14030023.
[33] С.С. Ставицкая, О.И. Поддубная, Н.Н. Цыба, А.М. Пузий, Каталитические свойства фосфорсодержащих углей в реакции гидролиза этилацетата, Теоретическая и Экспериментальная Химия. 50 (2014) 185–189.
[34] С.С. Ставицкая, В.М. Викарчук, М.Ф. Ковтун, О.И. Поддубная, А.М. Пузий, Адсорбция ионов меди углеродными адсорбентами, модифицированными фосфорной кислотой при различных температурах, Химия и Технология Воды. 36 (2014) 203–210.
[35] А.М. Пузий, С.С. Ставицкая, В.М. Викарчук, О.И. Поддубная, В.В. Волынец, Н.Н. Цыба, Фосфорсодержащие активные угли из кокосового ореха, их получение и структурно-сорбционные свойства, Український Хімічний Журнал. 80 (2014) 25–31.
[36] О.М. Пузій, Б.К. Пасальський, Н.Ю. Чикун, Розробка та вдосконалення вуглецевих сорбентів для очистки води, Інтегроване Управління Водними Ресурсами. 1 (2013) 287–294.
[37] N.I. Ermokhina, V.A. Nevinskiy, P.A. Manorik, V.G. Ilyin, V.N. Novichenko, M.M. Shcherbatiuk, D.O. Klymchuk, M.M. Tsyba, A.M. Puziy, Synthesis and characterization of thermally stable large-pore mesoporous nanocrystalline anatase, J. Solid State Chem. 200 (2013) 90–98. https://doi.org/10.1016/j.jssc.2012.12.034.
[38] A.M. Puziy, O.I. Poddubnaya, T.Y. Gromovoy, Laser desorption/ionization time of flight mass spectrometry of phosphorus-containing carbons, Carbon. 53 (2013) 405–408. https://doi.org/10.1016/j.carbon.2012.10.064.
[39] A.M. Puziy, O.I. Poddubnaya, M. Sobiesiak, B. Gawdzik, Structural and surface heterogeneity of phosphorus-containing polyimide-derived carbons: effect of heat treatment temperature, Adsorption. 19 (2013) 717–722. https://doi.org/10.1007/s10450-013-9497-4.
[40] N.I. Ermokhina, V.A. Nevinskiy, P.A. Manorik, V.G. Ilyin, N.N. Shcherbatyuk, D.O. Klymchyuk, A.M. Puziy, Synthesis of large-pore mesoporous nanocrystalline TiO2 microspheres, Mater. Lett. 75 (2012) 68–70. https://doi.org/10.1016/j.matlet.2012.01.133.
[41] N.V. Sych, S.I. Trofymenko, O.I. Poddubnaya, M.M. Tsyba, V.I. Sapsay, D.O. Klymchuk, A.M. Puziy, Porous structure and surface chemistry of phosphoric acid activated carbon from corncob, Appl. Surf. Sci. 261 (2012) 75–82. https://doi.org/10.1016/j.apsusc.2012.07.084.
[42] A.M. Puzii, S.S. Stavitskaya, O.I. Poddubnaya, V.M. Vikarchuk, N.N. Tsyba, Structural and adsorption properties of active carbon from coconut shells modified with phosphorus heteroatoms, Theor. Exp. Chem. 48 (2012) 272–277. https://doi.org/10.1007/s11237-012-9272-8.
[43] А.М. Пузий, С.С. Ставицкая, О.И. Поддубная, В.М. Викарчук, Н.Н. Цыба, Структурно-сорбционные свойства активных углей из кокосового ореха, модифицированных гетероатомами фосфора, Теоретическая и Экспериментальная Химия. 48 (2012) 252–256.
[44] Н.И. Ермохина, В.А. Невинский, П.А. Манорик, В.Г. Ильин, Н.Н. Цыба, А.М. Пузий, Н.Н. Щербатюк, Д.А. Климчук, Синтез нанотрубок из мезопористого нанокристаллического диоксида титана, Український Фізичний Журнал. 57 (2012) 763–768.
[45] N.I. Ermokhina, V.A. Nevinskiy, P.A. Manorik, V.G. Ilyin, N.N. Tsyba, A.M. Puziy, N.N. Shcherbatyuk, D.O. Klymchyuk, Synthesis of nanotubes from mesoporous nanocrystalline titanium dioxide, Ukr. J. Phys. 57 (2012) 761–766.
[46] О.М. Пузій, О.І. Піддубна, Кислотно-основнi властивостi фосфоровмiсних вуглецевих адсорбентiв, Український Хімічний Журнал. 78 (2012) 80–88.
[47] M. Sobiesiak, B. Gawdzik, A.M. Puziy, O.I. Poddubnaya, Thermal properties of porous copolymers of BM-DVB and their carbonization products, New Carbon Mater. 26 (2011) 137–144. https://doi.org/10.1016/S1872-5805(11)60072-3.
[48] Н.В. Сыч, С.И. Трофименко, А.М. Пузий, С.С. Ставицкая, Н.Н. Цыба, М.Ф. Ковтун, Поглощение техногенных загрязнителей активированными углями из лигноцеллюлозного сырья, Экотехнологии и Ресурсосбережение. (2011) 62–65.
[49] С.И. Трофименко, Н.В. Сыч, А.М. Пузий, Н.Н. Цыба, Развитие пористой структуры в процессе химического активирования кизиловой косточки ортофосфорной кислотой, Український Хімічний Журнал. 77 (2011) 99–102.
[50] Н.В. Сыч, С.И. Трофименко, В.М. Викарчук, А.М. Пузий, З. Акташ, Э. Ягмур, М.Ф. Ковтун, Сорбция ионов тяжелых металлов активными углями, полученными химическим активированием кизиловой косточки, Хімія, Фізика Та Технологія Поверхні. 2 (2011) 213–218. https://www.cpts.com.ua/index.php/cpts/article/view/91.
[51] А.М. Пузий, Способы получения, структура и физико-химические свойства фосфорилированных углеродных адсорбентов, Теоретическая и Экспериментальная Химия. 47 (2011) 265–278.
[52] A.M. Puzii, Methods of production, structure, and physicochemical characteristics of phosphorylated carbon adsorbents, Theor. Exp. Chem. 47 (2011) 277–291. https://doi.org/10.1007/s11237-011-9216-8.
[53] N.I. Yermokhina, V.K. Bukhtiyarov, Y.V. Kishenya, V.G. Illin, P.A. Manorik, L.M. Kapitanchuk, O.D. Smiyan, A.M. Puziy, D.S. Kamenskih, V.A. Bortyshevskyy, Nanocomposite Ni/TiO2-materials for hydrogen generation systems, Int. J. Hydrogen Energy. 36 (2011) 1364–1368. https://doi.org/10.1016/j.ijhydene.2010.06.131.
[54] A.M. Puziy, O.I. Poddubnaya, C.A. Reinish, M.M. Tsyba, L.I. Mikhalovska, S. V. Mikhalovsky, One-pot preparation of functionalized nanostructured carbons, Carbon. 49 (2011) 599–604. https://doi.org/10.1016/j.carbon.2010.10.002.
[55] M. Sobiesiak, B. Gawdzik, A.M. Puziy, O.I. Poddubnaya, Thermal properties of porous copolymers of BM-DVB and their carbonization products, Carbon. 49 (2011) 3707. https://doi.org/10.1016/j.carbon.2011.04.033.
[56] A.M. Puziy, O.I. Poddubnaya, B. Gawdzik, M. Sobiesiak, C.A. Reinish, M.M. Tsyba, T.P. Segeda, M.I. Danylenko, Nanostructured carbons for solid phase extraction, Appl. Surf. Sci. 256 (2010) 5216–5220. https://doi.org/10.1016/j.apsusc.2009.12.106.
[57] A.M. Puziy, O.I. Poddubnaya, V.N. Zaitsev, A bibasic method for investigation of the mechanism of heavy metal ion adsorption on heterogeneous adsorbents, Reports Natl. Acad. Sci. Ukr. (2010) 119–125.
[58] О.М. Пузій, О.І. Піддубна, В.М. Зайцев, Двобазисний метод дослідження механізму адсорбції іонів важких металів на неоднорідних адсорбентах, Доповіді Національної академії наук України. (2010) 119–125.
[59] M. Sobiesiak, B. Gawdzik, A.M. Puziy, O.I. Poddubnaya, Analysis of structure and properties of active carbons and their copolymeric precursors, Appl. Surf. Sci. 256 (2010) 5355–5360. https://doi.org/10.1016/j.apsusc.2009.12.077.
[60] A.M. Puziy, O.I. Poddubnaya, Y.N. Kochkin, N. V. Vlasenko, M.M. Tsyba, Acid properties of phosphoric acid activated carbons and their catalytic behavior in ethyl-tert-butyl ether synthesis, Carbon. 48 (2010) 706–713. https://doi.org/10.1016/j.carbon.2009.10.015.
[61] Н.В. Сыч, В.В. Стрелко, Н.Н. Цыба, А.М. Пузий, Влияние количества ортофосфорной кислоты на развитие пористой структуры углей при химическом активировании кукурузных кочерыжек, Доповіді Національної Академії Наук України. (2009) 144–148.
[62] D. Hulicova-Jurcakova, A.M. Puziy, O.I. Poddubnaya, F. Suárez-García, J.M.D. Tascón, G.Q. Lu, Highly stable performance of supercapacitors from phosphorus-enriched carbons, J. Am. Chem. Soc. 131 (2009) 5026–5027. https://doi.org/10.1021/ja809265m.
[63] A.M. Puziy, O.I. Poddubnaya, B. Gawdzik, M. Sobiesiak, C.A. Reinish, M.M. Tsyba, T.P. Segeda, M.I. Danylenko, Preparation of nanostructured carbons for solid phase extraction, Ann. UMCS, Chem. 64 (2009) 64–74. https://doi.org/10.2478/v10063-008-0006-7.
[64] A.M. Puziy, O.I. Poddubnaya, A. Martínez-Alonso, F. Suárez-García, A. Castro-Muñiz, J.M.D. Tascón, Impact of the carbonization atmosphere on the properties of phosphoric acid-activated carbons from fruit stones, Adsorpt. Sci. Technol. 26 (2008) 843–851.
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